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The song was among his biggest hits, earning a gold record and reaching No. 2 on the Billboard Hot 100 for a week, stuck behind "Windy" by the Association. Gaudio was a bandmate of Valli's in the Four Seasons. It was Valli's biggest solo hit until he hit No. 1 in 1975 with "My Eyes Adored You". "Can't Take My Eyes Off You" has been recorded in many other arrangements, many of which have been on the charts in different countries. Franki Valli's version was used by NASA as a wake-up song on the STS-126 Space Shuttle mission, to celebrate the wedding anniversary of astronaut Christopher Ferguson, one of the mission's crew members.